1Introduction

Hiroyuki Fujiwara

Gifu University, Department of Electrical, Electronic and Computer Engineering, 1‐1 Yanagido, Gifu, 501‐1193, Japan

1.1 Hybrid Perovskite Solar Cells

Hybrid perovskites, unique materials composed of moving organic cations and rigid inorganic framework, show remarkable suitability as light absorbers of photovoltaic devices, enabling us to reach a 25% efficiency in a single‐cell configuration [1] and a 29% efficiency in a tandem device configuration [1] in a rather short period of time since the first development of a hybrid perovskite solar cell in 2009 [2]. Compared with structurally complex solar cells such as Si [3, 4], GaAs [5], and CuInGaSe2 [3, 6], the architecture of hybrid perovskite solar cells is surprisingly ...

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