
Zero Area Pulse Propagation 515
Recent advances in fs photon echo spectroscopy of molecules and solids are
summarized in papers by Ashbury et al. [20] and Dao et al. [21].
In summary, the photon echo method is quite powerful and useful for the
determination of relaxation times longer than the pulse duration. It has been one
of the most commonly used.
10.9. ZERO AREA PULSE PROPAGATION
The photon echo experiment is based on a sequence of two nonoverlapping
pulses whose relative phase is unimportant. An essential feature of coherent exci-
tation is that the excitation depends on the phase of the applied signal. We saw in
Chapter 4 that a sequence of two ...